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Flexible fiber-reinforced composites with improved interfacial adhesion by mussel-inspired polydopamine and poly(methyl methacrylate) coating
Yi, Mi1; Sun, Hongyang1; Zhang, Hongcheng1; Deng, Xuliang2; Cai, Qing1; Yang, Xiaoping1
关键词Fiber-reinforced Composite Prepreg Interfacial Adhesion Surface Modification Polydopamine Poly(Methyl Methacrylate)
刊名MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS
2016
DOI10.1016/j.msec.2015.09.026
58页:742-749
收录类别SCI
文章类型Article
WOS标题词Science & Technology
类目[WOS]Materials Science, Biomaterials
研究领域[WOS]Materials Science
关键词[WOS]SURFACE MODIFICATION ; RESTORATIVE COMPOSITE ; POLY(DOPAMINE) ; RESIN ; FUNCTIONALIZATION ; POLYMERIZATION ; NANOFIBERS ; STRENGTH ; SYSTEMS ; MATRIX
英文摘要

To obtain a kind of light-curable fiber-reinforced composite for dental restoration, an excellent interfacial adhesion between the fiber and the acrylate resin matrix is quite essential. Herein, surface modification on glass fibers were carried out by coating them with poly(methyl methacrylate) (PMMA), polydopamine (PDA), or both. The PMMA or PDA coating was performed by soaking fibers in PMMA/acetone solution or dopamine aqueous solution. PDA/PMMA co-coated glass fibers were obtained by further soaking PDA-coated fibers in PMMA/acetone solution. These modified fibers were impregnated with bisphenol A glycidyl methacrylate (Bis-GMA)/triethylene glycol dimethacrylate (TEGDMA) (5:5, w/w) dental resin at a volume fraction of 75%, using unmodified fibers as reference. Light-cured specimens were submitted to evaluations including flexural properties, morphological observation, dynamic mechanical thermal analysis (DMTA) and pull-out test. In comparison with unmodified glass fibers, all the modified glass fibers showed enhancements in flexural strength and modulus of Bis-GMA/TEGDMA resin composites. Results of DMTA and pull-out tests confirmed that surface modification had significantly improved the interfacial adhesion between the glass fiber and the resin matrix. Particularly, the PDA/PMMA co-coated glass fibers displayed the most efficient reinforcement and the strongest interfacial adhesion due to the synergetic effects of PDA and PMMA. It indicated that co-coating method was a promising approach in modifying the interfacial compatibility between inorganic glass fiber and organic resin matrix. (C) 2015 Elsevier B.V. All rights reserved.

语种英语
WOS记录号WOS:000364247500088
项目编号51373016 ; ZDZH20141001001
资助机构National Natural Science Foundation of China ; Beijing Municipal Commission of Education
引用统计
被引频次:13[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.bjmu.edu.cn/handle/400002259/53271
专题北京大学口腔医学院
北京大学口腔医学院_特诊科
作者单位1.Beijing Univ Chem Technol, Being Lab Biomed Mat, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
2.Peking Univ, Dept Geriatr Dent, Sch & Hosp Stomatol, Beijing 100081, Peoples R China
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GB/T 7714
Yi, Mi,Sun, Hongyang,Zhang, Hongcheng,et al. Flexible fiber-reinforced composites with improved interfacial adhesion by mussel-inspired polydopamine and poly(methyl methacrylate) coating[J]. MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS,2016,58:742-749.
APA Yi, Mi,Sun, Hongyang,Zhang, Hongcheng,Deng, Xuliang,Cai, Qing,&Yang, Xiaoping.(2016).Flexible fiber-reinforced composites with improved interfacial adhesion by mussel-inspired polydopamine and poly(methyl methacrylate) coating.MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS,58,742-749.
MLA Yi, Mi,et al."Flexible fiber-reinforced composites with improved interfacial adhesion by mussel-inspired polydopamine and poly(methyl methacrylate) coating".MATERIALS SCIENCE & ENGINEERING C-MATERIALS FOR BIOLOGICAL APPLICATIONS 58(2016):742-749.
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