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Multiple Oxidative Dehydrogenative Functionalization of Arylacetaldehydes Using Molecular Oxygen as Oxidant Leading to 2-Oxo-acetamidines
Zhang, Chun1; Zhang, Liangren1; Jiao, Ning1,2
关键词Copper Cross-coupling Dehydrogenation Oxidation Oxygen
刊名ADVANCED SYNTHESIS & CATALYSIS
2012-05-01
DOI10.1002/adsc.201100892
354期:7页:1293-1300
收录类别SCI ; IC ; CCR
文章类型Review
WOS标题词Science & Technology
类目[WOS]Chemistry, Applied ; Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]C-H BOND ; COPPER-CATALYZED TRIFLUOROMETHYLATION ; CARBON-HYDROGEN BONDS ; TERMINAL ALKYNES ; N-HYDROXYPHTHALIMIDE ; DIOXYGEN ACTIVATION ; COUPLING REACTIONS ; ORTHO-BORYLATION ; PALLADIUM ; EFFICIENT
英文摘要

A novel copper-catalyzed, multiple oxidative dehydrogenative functionalization of arylacetaldehydes leading to 2-oxo-acetamidine compounds has been developed. This transformation is highly efficient with dissociation of six hydrogens including two sp3 C?H and one sp2 C?H bond activations. This method not only provides an efficient approach to 2-oxo-acetamidine compounds, but also offers a valuable mechanistic insight into this novel copper catalysis.

语种英语
WOS记录号WOS:000303495900010
项目编号20872003 ; 2009CB825300
资助机构Peking University ; National Science Foundation of China ; National Basic Research Program of China (973 Program)
引用统计
被引频次:23[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.bjmu.edu.cn/handle/400002259/53502
专题北京大学药学院
北京大学药学院_天然药物与仿生药物国家重点实验室
北京大学药学院_药物化学系
作者单位1.Peking Univ, Sch Pharmaceut Sci, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China
2.Chinese Acad Sci, State Key Lab Organometall Chem, Shanghai 200032, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Chun,Zhang, Liangren,Jiao, Ning. Multiple Oxidative Dehydrogenative Functionalization of Arylacetaldehydes Using Molecular Oxygen as Oxidant Leading to 2-Oxo-acetamidines[J]. ADVANCED SYNTHESIS & CATALYSIS,2012,354(7):1293-1300.
APA Zhang, Chun,Zhang, Liangren,&Jiao, Ning.(2012).Multiple Oxidative Dehydrogenative Functionalization of Arylacetaldehydes Using Molecular Oxygen as Oxidant Leading to 2-Oxo-acetamidines.ADVANCED SYNTHESIS & CATALYSIS,354(7),1293-1300.
MLA Zhang, Chun,et al."Multiple Oxidative Dehydrogenative Functionalization of Arylacetaldehydes Using Molecular Oxygen as Oxidant Leading to 2-Oxo-acetamidines".ADVANCED SYNTHESIS & CATALYSIS 354.7(2012):1293-1300.
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