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Relay Catalysis by a Multifunctional Cu Catalyst in a Tandem Dehydro-/Dehalogenation Sequence along with N-Arylation
Liang, Lei; Wang, Wei; Xu, Fengrong; Niu, Yan; Sun, Qi; Xu, Ping
刊名ORGANIC LETTERS
2013-06-07
DOI10.1021/ol401105x
15期:11页:2770-2773
收录类别SCI ; IC ; CCR
文章类型Article
WOS标题词Science & Technology
类目[WOS]Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]CARBON-HALOGEN BOND ; NOBLE-METAL SALTS ; AEROBIC DEHYDROGENATION ; ORGANIC HALIDES ; COUPLING REACTIONS ; HYDROGEN TRANSFER ; ARYL CHLORIDES ; AQUEOUS-MEDIA ; WATER ; DEHALOGENATION
英文摘要

A Cu-catalyzed tandem dehydrogenation/dehalogenation sequential reaction along with N-arylation has been developed for the synthesis of pyridazinone derivatives in an aerobic and aqueous environment. To achieve the transformation of three chemical bonds in a one-pot reaction, a multifunctional copper catalyst was used which afforded excellent activity, high selectivity, and recyclability. The catalytic system consists of a water-soluble Cusalen complex and Na2CO3 in neat water and an air atmosphere.

语种英语
WOS记录号WOS:000320298900052
项目编号7112088 ; 2012CB518000 ; 21202003/21172012
资助机构Beijing Natural Science Foundation ; National Basic Research Program of China ; National Natural Science Foundation of China
引用统计
被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.bjmu.edu.cn/handle/400002259/58122
专题北京大学药学院_药物化学系
北京大学药学院_化学生物学系
作者单位Peking Univ Hlth Sci Ctr, Sch Pharmaceut Sci, Dept Med Chem, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China
推荐引用方式
GB/T 7714
Liang, Lei,Wang, Wei,Xu, Fengrong,et al. Relay Catalysis by a Multifunctional Cu Catalyst in a Tandem Dehydro-/Dehalogenation Sequence along with N-Arylation[J]. ORGANIC LETTERS,2013,15(11):2770-2773.
APA Liang, Lei,Wang, Wei,Xu, Fengrong,Niu, Yan,Sun, Qi,&Xu, Ping.(2013).Relay Catalysis by a Multifunctional Cu Catalyst in a Tandem Dehydro-/Dehalogenation Sequence along with N-Arylation.ORGANIC LETTERS,15(11),2770-2773.
MLA Liang, Lei,et al."Relay Catalysis by a Multifunctional Cu Catalyst in a Tandem Dehydro-/Dehalogenation Sequence along with N-Arylation".ORGANIC LETTERS 15.11(2013):2770-2773.
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