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学科主题: 药学
题名:
Relay Catalysis by a Multifunctional Cu Catalyst in a Tandem Dehydro-/Dehalogenation Sequence along with N-Arylation
作者: Liang, Lei; Wang, Wei; Xu, Fengrong; Niu, Yan; Sun, Qi; Xu, Ping
刊名: ORGANIC LETTERS
发表日期: 2013-06-07
DOI: 10.1021/ol401105x
卷: 15, 期:11, 页:2770-2773
收录类别: SCI ; IC ; CCR
文章类型: Article
WOS标题词: Science & Technology
类目[WOS]: Chemistry, Organic
研究领域[WOS]: Chemistry
关键词[WOS]: CARBON-HALOGEN BOND ; NOBLE-METAL SALTS ; AEROBIC DEHYDROGENATION ; ORGANIC HALIDES ; COUPLING REACTIONS ; HYDROGEN TRANSFER ; ARYL CHLORIDES ; AQUEOUS-MEDIA ; WATER ; DEHALOGENATION
英文摘要:

A Cu-catalyzed tandem dehydrogenation/dehalogenation sequential reaction along with N-arylation has been developed for the synthesis of pyridazinone derivatives in an aerobic and aqueous environment. To achieve the transformation of three chemical bonds in a one-pot reaction, a multifunctional copper catalyst was used which afforded excellent activity, high selectivity, and recyclability. The catalytic system consists of a water-soluble Cusalen complex and Na2CO3 in neat water and an air atmosphere.

语种: 英语
所属项目编号: 7112088 ; 2012CB518000 ; 21202003/21172012
项目资助者: Beijing Natural Science Foundation ; National Basic Research Program of China ; National Natural Science Foundation of China
WOS记录号: WOS:000320298900052
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.bjmu.edu.cn/handle/400002259/58122
Appears in Collections:北京大学药学院_药物化学系_期刊论文

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作者单位: Peking Univ Hlth Sci Ctr, Sch Pharmaceut Sci, Dept Med Chem, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China

Recommended Citation:
Liang, Lei,Wang, Wei,Xu, Fengrong,et al. Relay Catalysis by a Multifunctional Cu Catalyst in a Tandem Dehydro-/Dehalogenation Sequence along with N-Arylation[J]. ORGANIC LETTERS,2013,15(11):2770-2773.
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