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Csp(2)-Csp(2) bond formation via Lewis acid/ammonium salt cocatalyzed tandem addition and oxidative dehydrogenation strategy: alkenylation of indoles with alpha,beta-unsaturated ketones
Xiang, Shi-Kai2; Wu, Guolin1; Zhang, Bo1; Cui, Yuxin1; Jiao, Ning1,3
关键词Alkenylation Indoles alpha,beta-Unsaturated ketones Tandem reaction Lewis acids Organocatalyst
刊名TETRAHEDRON LETTERS
2012-07-18
DOI10.1016/j.tetlet.2012.05.053
53期:29页:3802-3804
收录类别SCI ; IC ; CCR
文章类型Article
WOS标题词Science & Technology
类目[WOS]Chemistry, Organic
研究领域[WOS]Chemistry
关键词[WOS]C-H FUNCTIONALIZATION ; ASYMMETRIC ENAMINE CATALYSIS ; DIRECT C-2 ARYLATION ; ROOM-TEMPERATURE ; PALLADIUM ; PYRROLES ; ALDEHYDES ; CYCLIZATION ; REGIOSELECTIVITY ; ACIDS
英文摘要

The alkenylation of indoles with alpha,beta-unsaturated ketones through a tandem addition and oxidative dehydrogenation strategy has been developed. This method provides an alternative approach for C3 alkenylation of indoles with alpha,beta-unsaturated ketones. Using inexpensive and readily available BF3 center dot Et2O and an ammonium salt as the efficient cocatalyst constitutes the attractive advantage of this reaction. (C) 2012 Published by Elsevier Ltd.

语种英语
WOS记录号WOS:000306027700028
项目编号2009CB825300 ; 20872003 ; 21172006
资助机构National Basic Research Program of China (973 Program) ; National Science Foundation of China ; Peking University
引用统计
被引频次:9[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.bjmu.edu.cn/handle/400002259/60036
专题北京大学药学院
北京大学药学院_天然药物与仿生药物国家重点实验室
作者单位1.Perking Univ, Sch Pharmaceut Sci, Peking Univ, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China
2.Sichuan Normal Univ, Coll Chem & Mat Sci, Chengdu 610066, Sichuan, Peoples R China
3.E China Normal Univ, Dept Chem, Shanghai Key Lab Green Chem & Chem Proc, Shanghai 200062, Peoples R China
推荐引用方式
GB/T 7714
Xiang, Shi-Kai,Wu, Guolin,Zhang, Bo,et al. Csp(2)-Csp(2) bond formation via Lewis acid/ammonium salt cocatalyzed tandem addition and oxidative dehydrogenation strategy: alkenylation of indoles with alpha,beta-unsaturated ketones[J]. TETRAHEDRON LETTERS,2012,53(29):3802-3804.
APA Xiang, Shi-Kai,Wu, Guolin,Zhang, Bo,Cui, Yuxin,&Jiao, Ning.(2012).Csp(2)-Csp(2) bond formation via Lewis acid/ammonium salt cocatalyzed tandem addition and oxidative dehydrogenation strategy: alkenylation of indoles with alpha,beta-unsaturated ketones.TETRAHEDRON LETTERS,53(29),3802-3804.
MLA Xiang, Shi-Kai,et al."Csp(2)-Csp(2) bond formation via Lewis acid/ammonium salt cocatalyzed tandem addition and oxidative dehydrogenation strategy: alkenylation of indoles with alpha,beta-unsaturated ketones".TETRAHEDRON LETTERS 53.29(2012):3802-3804.
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