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Direct Transformation of N,N-Dimethylformamide to -CN: Pd-Catalyzed Cyanation of Heteroarenes via C-H Functionalization
Ding, Shengtao1; Jiao, Ning1,2
刊名JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
2011-08-17
DOI10.1021/ja204063z
133期:32页:12374-12377
收录类别SCI ; IC ; CCR
文章类型Article
WOS标题词Science & Technology
类目[WOS]Chemistry, Multidisciplinary
资助者Peking University ; National Natural Science Foundation of China ; National Basic Research Program of China (973 Program) ; Peking University ; National Natural Science Foundation of China ; National Basic Research Program of China (973 Program)
研究领域[WOS]Chemistry
关键词[WOS]ONE-POT CONVERSION ; ARYL HALIDES ; TERTIARY-AMINES ; OXIDATIVE CONVERSION ; MOLECULAR-OXYGEN ; CORRESPONDING NITRILES ; HETEROGENEOUS CATALYST ; AEROBIC CONDITIONS ; ALKENYL NITRILES ; CYANIDE SOURCE
英文摘要

This paper describes the direct cyanation of indoles and benzofurans employing N,N-dimethylformamide (DMF) as both reagent and solvent. Isotopic labeling experiments indicated that both the N and the C of the cyano group derived from DMF. This transformation offers an alternative method for preparing aryl nitriles, though it is currently limited in scope to indoles and benzofurans.

语种英语
所属项目编号20702002 ; 20872003 ; 2009CB825300
资助者Peking University ; National Natural Science Foundation of China ; National Basic Research Program of China (973 Program) ; Peking University ; National Natural Science Foundation of China ; National Basic Research Program of China (973 Program)
WOS记录号WOS:000294740000015
引用统计
被引频次:195[WOS]   [WOS记录]     [WOS相关记录]
文献类型期刊论文
条目标识符http://ir.bjmu.edu.cn/handle/400002259/64179
专题北京大学药学院
作者单位1.Peking Univ, Sch Pharmaceut Sci, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China
2.Chinese Acad Sci, State Key Lab Organometall Chem, Shanghai 200032, Peoples R China
推荐引用方式
GB/T 7714
Ding, Shengtao,Jiao, Ning. Direct Transformation of N,N-Dimethylformamide to -CN: Pd-Catalyzed Cyanation of Heteroarenes via C-H Functionalization[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,2011,133(32):12374-12377.
APA Ding, Shengtao,&Jiao, Ning.(2011).Direct Transformation of N,N-Dimethylformamide to -CN: Pd-Catalyzed Cyanation of Heteroarenes via C-H Functionalization.JOURNAL OF THE AMERICAN CHEMICAL SOCIETY,133(32),12374-12377.
MLA Ding, Shengtao,et al."Direct Transformation of N,N-Dimethylformamide to -CN: Pd-Catalyzed Cyanation of Heteroarenes via C-H Functionalization".JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 133.32(2011):12374-12377.
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