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学科主题: 药学
题名:
Copper-Catalyzed Aerobic Oxidative C-C Bond Cleavage for C-N Bond Formation: From Ketones to Amides
作者: Tang, Conghui1; Jiao, Ning1,2
关键词: amides ; cleavage reactions ; copper ; ketones ; oxygen
刊名: ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
发表日期: 2014-06-01
DOI: 10.1002/anie.201403528
卷: 53, 期:25, 页:6528-6532
收录类别: SCI ; CCR
文章类型: Article
WOS标题词: Science & Technology
类目[WOS]: Chemistry, Multidisciplinary
研究领域[WOS]: Chemistry
关键词[WOS]: ALPHA-HYDROXYPHENYLACETIC ACIDS ; CARBON TRIPLE BOND ; ARYL ALKYL KETONES ; MOLECULAR-OXYGEN ; METAL-FREE ; ROOM-TEMPERATURE ; DIRECT TRANSFORMATION ; PHENYLACETIC ACIDS ; ALCOHOL OXIDATIONS ; ORGANIC-CHEMICALS
英文摘要:

A novel copper-catalyzed aerobic oxidative C(CO)-C(alkyl) bond cleavage reaction of aryl alkyl ketones for C-N bond formation is described. A series of acetophenone derivatives as well as more challenging aryl ketones with long-chain alkyl substituents could be selectively cleaved and converted into the corresponding amides, which are frequently found in biologically active compounds and pharmaceuticals.

语种: 英语
所属项目编号: 21325206 ; 21172006 ; 20120001110013
项目资助者: National Science Foundation of China ; National Young Top-notch Talent Support Program ; Ph.D. Programs Foundation of the Ministry of Education of China
WOS记录号: WOS:000337095900040
Citation statistics:
内容类型: 期刊论文
URI标识: http://ir.bjmu.edu.cn/handle/400002259/65274
Appears in Collections:北京大学药学院_期刊论文

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作者单位: 1.Peking Univ, Sch Pharmaceut Sci, State Key Lab Nat & Biomimet Drugs, Beijing 100191, Peoples R China
2.Chinese Acad Sci, State Key Lab Organometall Chem, Shanghai 200032, Peoples R China

Recommended Citation:
Tang, Conghui,Jiao, Ning. Copper-Catalyzed Aerobic Oxidative C-C Bond Cleavage for C-N Bond Formation: From Ketones to Amides[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2014,53(25):6528-6532.
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